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Pat the chuck roast pieces dry with paper towels and season all over with the salt and black pepper.
Heat the vegetable oil in a 12-inch skillet over medium-high heat until shimmering. Add the beef pieces in a single layer — work in two batches if needed to avoid crowding — and sear undisturbed for 3–4 minutes per side, until a deep brown crust forms on each surface. Transfer the seared pieces to the slow cooker insert.
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