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In a small bowl, combine the smoked paprika, garlic powder, onion powder, cumin, salt, black pepper, and cayenne. Pat the pork shoulder chunks dry with paper towels, then rub the spice mixture evenly over all sides of each piece.
Select the Sauté function on the Instant Pot and add the olive oil. Once the oil is shimmering, add the pork chunks in a single layer (work in two batches if needed to avoid crowding) and sear for 3–4 minutes per side, until deeply browned on at least two sides. Transfer the seared pork to a plate and repeat with any remaining pieces.
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